kaz44Вестник Университета Шакарима. Серия технические наукиBulletin of Shakarim University. Technical Sciences2788-79953006-0524«Шәкәрім университеті» КеАҚ10.53360/2788-7995-2024-2(14)-58kaz44-754Research ArticleХИМИЧЕСКАЯ ТЕХНОЛОГИЯ (ОРИГИНАЛЬНАЯ СТАТЬЯ)CHEMICAL TECHNOLOGY (ORIGINAL ARTICLE)ЭКСТРАКЦИОННАЯ СЕРООЧИСТКА НЕФТЯНОГО ТОПЛИВА С ИСПОЛЬЗОВАНИЕМ ГЛУБОКОЭВТЕКТИЧЕСКИХ РАСТВОРИТЕЛЕЙEXTRACTIVE DESULFURIZATIONOF PETROLEUM FUEL USING DEEP-EUTECTIC SOLVENTShttps://orcid.org/0000-0002-4167-8921КеримкуловаА. Ж.KerimkulovaA. Zh.

Айгуль Жадраевна Керимкулова – Кандидат химических наук, ассоциированный профессор кафедры ХиБИ 

050013, Республика Казахстан, г. Алматы, ул. Сатпаева 22 а 

Aigul Zhadraevna Kerimkulova – Candidate of Chemical Sciences, Associate Professor 

050013, Republic of Kazakhstan, Almaty,22 Satbayev Street 

kerimkulova07@mail.ruhttps://orcid.org/0000-0001-8028-2244РафиковаХ. С.RafikovaKh. S.

Хадичахан Сабыржановна Рафикова – PhDДоктор, ассоциированный профессор кафедры ХиБИ

050013, Республика Казахстан, г. Алматы, ул. Сатпаева 22 а 

Khadichakhan Sabrzhanovna Rafikova – PhD in Petrochemistry, Associate professor 

050013, Republic of Kazakhstan, Almaty,22 Satbayev Street 

kh.rafikova@satbayev.universityhttps://orcid.org/0009-0003-9698-2562БулатоваН. Б.BulatovaN. B.

Нурлыару Булатовна Булатова – магистрант, Satbayev University, г. Алматы, РеспубликаКазахстан; е-mail:  

050013, Республика Казахстан, г. Алматы, ул. Сатпаева 22 а 

Nurlyaru Bulatovna Bulatova – мaster student 

050013, Republic of Kazakhstan, Almaty,22 Satbayev Street 

nurlyaru02@gmail.comАбдирафиеваД. О.AbdirafiyevaD. O.

Диана Олеговна Абдирафиева – магистрант

050013, Республика Казахстан, г. Алматы, ул. Сатпаева 22 а 

Diana Olegovna Abdirafiyeva – мaster student

050013, Republic of Kazakhstan, Almaty,22 Satbayev Street 

diabdirafieva@mail.ruhttps://orcid.org/0009-0003-1733-0380ДариджанМ. Е.DaridzhanM. E.

Мадина Еркінқызы Дариджан – магистрант

050013, Республика Казахстан, город Алматы, ул. Толе би, 100 

Madina Erkinkyzy Daridzhan – мaster student 

050012, Republic of Kazakhstan, Almaty,100 Tole bi Street 

madina.daridzhan@mail.ruКазНИТУ имени К.И.СатпаеваКазахстанSatbayev UniversityKazakhstanАлматинский технологический университетAlmaty Technological University20242906202412(14)481495Copyright © Керимкулова А.Ж., Рафикова Х.С., Булатова Н.Б., Абдирафиева Д.О., Дариджан М.Е., 20242024Керимкулова А.Ж., Рафикова Х.С., Булатова Н.Б., Абдирафиева Д.О., Дариджан М.Е.Kerimkulova A.Z., Rafikova K.S., Bulatova N.B., Abdirafiyeva D.O., Daridzhan M.E.Данная работа распространяется под лицензией Creative Commons Attribution 4.0.This work is licensed under a Creative Commons Attribution 4.0 License.https://tech.vestnik.shakarim.kz/jour/article/view/754

В ближайшие десятилетия невозможно недооценить важность создания экологически чистой энергетики и связанных с ней применений. Доказано, что минимизация и устранение токсичных выбросов имеют решающее значение для выживания нашей планеты. Соединения серы (S) в топливе приводят к образованию токсичных выбросов, представляющих серьезную угрозу для окружающей среды. Поэтому во всем мире активизировались исследования процесса сероочистки для получения топлива с низким содержанием S. Традиционная технология гидродесульфуризации (HDS) не получила широкого распространения из-за ряда недостатков, таких как высокая стоимость, повышенное потребление электроэнергии, повышенное образование водорода и использование катализаторов с высоким содержанием благородных металлов. Перспективной альтернативой HDS является процесс экстрактивной сероочистки (EDS) благодаря мягким условиям эксплуатации. В последние годы большое внимание в исследованиях уделяется использованию глубокоэвтектических растворителей (DES), образующихся из эвтектической смеси кислот и оснований Льюиса/Бренстеда.Целью данного обзора является обсуждение преимуществ EDS с использованием DES по сравнению с другими методами сероочистки, а также описание различных факторов сероочистки, таких как природа DES, массовое соотношение DES и топлива, температура, взаимная растворимость, время, начальное содержание S. Потенциальные проблемы и недостатки EDS с использованием DES изучены достаточно полно. В данном обзоре обсуждаются вопросы применения DES в качестве экстрагентов для получения экологически чистого топлива вместо традиционных органических растворителей. Необходимость обозревания исследований по данной тематики исходит из актуальности поиска более экологически чистых соединений, соответствующих всем принципам «зеленой химии». В обзоре рассмотрены исследования за последние 10-20 лет в области применения DES в качестве экстрагентов для очистки топлив от серосоединений.

In the coming decades, the importance of creating clean energy and its associated applications cannot be underestimated. Minimizing and eliminating toxic emissions has been proven to be critical to the survival of our planet. Sulfur (S) compounds in fuel create toxic emissions that pose a serious threat to the environment. Therefore, research on the desulphurization process has intensified worldwide to produce fuels with low S content. Traditional hydrodesulfurization (HDS) technology has not been widely adopted due to several disadvantages such as high cost, increased energy consumption, increased hydrogen production and the use of high content catalysts noble metals. A promising alternative to HDS is the extractive desulfurization (EDS) process due to its mild operating conditions. In recent years, much research attention has been paid to the use of deep eutectic solvents (DES), formed from a eutectic mixture of Lewis/Brønsted acids and bases. The purpose of this review is to discuss the advantages of EDS using DES compared to other desulfurization methods, as well as to describe various desulfurization factors such as the nature of DES, mass ratio of DES to fuel, temperature, mutual solubility, time, initial S content. The potential problems and shortcomings of EDS using DES have been well studied. Due to the promising physicochemical properties of DES, this review recommends DES as a preferred candidate over many molecular organic solvents in the field of clean petroleum fuel production.

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The authors declare that there are no conflicts of interest present.